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Evaporate-casting of curvature gradient graphene superstructures for ultra-high strength structural materials

Bing Lu, Li Yu, Yajie Hu, Ying Wang, Fei Zhao, Yang Zhao (), Feng Liu (), Huhu Cheng and Liangti Qu ()
Additional contact information
Bing Lu: Ministry of Education, Tsinghua University
Li Yu: Institute of Mechanics, Chinese Academy of Sciences
Yajie Hu: Ministry of Education, Tsinghua University
Ying Wang: Ministry of Education, Tsinghua University
Fei Zhao: School of Chemistry and Chemical Engineering, Beijing Institute of Technology
Yang Zhao: School of Chemistry and Chemical Engineering, Beijing Institute of Technology
Feng Liu: Institute of Mechanics, Chinese Academy of Sciences
Huhu Cheng: Ministry of Education, Tsinghua University
Liangti Qu: Ministry of Education, Tsinghua University

Nature Communications, 2024, vol. 15, issue 1, 1-10

Abstract: Abstract In contemporary manufacturing, the processing of structural materials plays a pivotal role in enabling the creation of robust, tailor-made, and precise components suitable for diverse industrial applications. Nonetheless, current material forming technologies face challenges due to internal stress and defects, resulting in a substantial decline in both mechanical properties and processing precision. We herein develop a processing strategy toward graphene superstructure with a curvature gradient, which allows us to fabricate robust structural materials with meticulously designed functional shapes. The structure consists of an arc-shaped assembly of graphene nanosheets positioned at co-axial curvature centers. During the dehydration-based evaporate-casting process, the assembly is tightened via capillary effect, inducing local bending. By precisely tuning the axis-center distance and tilt angle, we achieve accurate control over the shape of obtained structure. Notably, internal stress is harnessed to reinforce a designed mortise and tenon structure, resulting in a high joining strength of up to ~200 MPa. This innovative approach addresses the challenges faced by current material forming technologies and opens up more possibilities for the manufacturing of robust and precisely shaped components.

Date: 2024
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DOI: 10.1038/s41467-024-50191-6

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