Evaporate-casting of curvature gradient graphene superstructures for ultra-high strength structural materials
Bing Lu,
Li Yu,
Yajie Hu,
Ying Wang,
Fei Zhao,
Yang Zhao (),
Feng Liu (),
Huhu Cheng and
Liangti Qu ()
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Bing Lu: Ministry of Education, Tsinghua University
Li Yu: Institute of Mechanics, Chinese Academy of Sciences
Yajie Hu: Ministry of Education, Tsinghua University
Ying Wang: Ministry of Education, Tsinghua University
Fei Zhao: School of Chemistry and Chemical Engineering, Beijing Institute of Technology
Yang Zhao: School of Chemistry and Chemical Engineering, Beijing Institute of Technology
Feng Liu: Institute of Mechanics, Chinese Academy of Sciences
Huhu Cheng: Ministry of Education, Tsinghua University
Liangti Qu: Ministry of Education, Tsinghua University
Nature Communications, 2024, vol. 15, issue 1, 1-10
Abstract:
Abstract In contemporary manufacturing, the processing of structural materials plays a pivotal role in enabling the creation of robust, tailor-made, and precise components suitable for diverse industrial applications. Nonetheless, current material forming technologies face challenges due to internal stress and defects, resulting in a substantial decline in both mechanical properties and processing precision. We herein develop a processing strategy toward graphene superstructure with a curvature gradient, which allows us to fabricate robust structural materials with meticulously designed functional shapes. The structure consists of an arc-shaped assembly of graphene nanosheets positioned at co-axial curvature centers. During the dehydration-based evaporate-casting process, the assembly is tightened via capillary effect, inducing local bending. By precisely tuning the axis-center distance and tilt angle, we achieve accurate control over the shape of obtained structure. Notably, internal stress is harnessed to reinforce a designed mortise and tenon structure, resulting in a high joining strength of up to ~200 MPa. This innovative approach addresses the challenges faced by current material forming technologies and opens up more possibilities for the manufacturing of robust and precisely shaped components.
Date: 2024
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DOI: 10.1038/s41467-024-50191-6
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