Autonomous discovery of optically active chiral inorganic perovskite nanocrystals through an intelligent cloud lab
Jiagen Li,
Junzi Li,
Rulin Liu,
Yuxiao Tu,
Yiwen Li,
Jiaji Cheng (),
Tingchao He () and
Xi Zhu ()
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Jiagen Li: The Chinese University of Hong Kong, Shenzhen (CUHK-Shenzhen)
Junzi Li: Shenzhen University
Rulin Liu: The Chinese University of Hong Kong, Shenzhen (CUHK-Shenzhen)
Yuxiao Tu: The Chinese University of Hong Kong, Shenzhen (CUHK-Shenzhen)
Yiwen Li: Hubei University
Jiaji Cheng: Hubei University
Tingchao He: Shenzhen University
Xi Zhu: The Chinese University of Hong Kong, Shenzhen (CUHK-Shenzhen)
Nature Communications, 2020, vol. 11, issue 1, 1-10
Abstract:
Abstract We constructed an intelligent cloud lab that integrates lab automation with cloud servers and artificial intelligence (AI) to detect chirality in perovskites. Driven by the materials acceleration operating system in cloud (MAOSIC) platform, on-demand experimental design by remote users was enabled in this cloud lab. By employing artificial intelligence of things (AIoT) technology, synthesis, characterization, and parameter optimization can be autonomously achieved. Through the remote collaboration of researchers, optically active inorganic perovskite nanocrystals (IPNCs) were first synthesized with temperature-dependent circular dichroism (CD) and inversion control. The inter-structure (structural patterns) and intra-structure (screw dislocations) dual-pattern-induced mechanisms detected by MAOSIC were comprehensively investigated, and offline theoretical analysis revealed the thermodynamic mechanism inside the materials. This self-driving cloud lab enables efficient and reliable collaborations across the world, reduces the setup costs of in-house facilities, combines offline theoretic analysis, and is practical for accelerating the speed of material discovery.
Date: 2020
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DOI: 10.1038/s41467-020-15728-5
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