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Intrinsic supercurrent non-reciprocity coupled to the crystal structure of a van der Waals Josephson barrier

Jae-Keun Kim (), Kun-Rok Jeon, Pranava K. Sivakumar, Jaechun Jeon, Chris Koerner, Georg Woltersdorf and Stuart S. P. Parkin ()
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Jae-Keun Kim: Max Planck Institute of Microstructure Physics, Weinberg 2
Kun-Rok Jeon: Chung-Ang University (CAU)
Pranava K. Sivakumar: Max Planck Institute of Microstructure Physics, Weinberg 2
Jaechun Jeon: Max Planck Institute of Microstructure Physics, Weinberg 2
Chris Koerner: Martin Luther University Halle-Wittenberg, Von-Danckelmann-Platz 3
Georg Woltersdorf: Martin Luther University Halle-Wittenberg, Von-Danckelmann-Platz 3
Stuart S. P. Parkin: Max Planck Institute of Microstructure Physics, Weinberg 2

Nature Communications, 2024, vol. 15, issue 1, 1-8

Abstract: Abstract Non-reciprocal electronic transport in a spatially homogeneous system arises from the simultaneous breaking of inversion and time-reversal symmetries. Superconducting and Josephson diodes, a key ingredient for future non-dissipative quantum devices, have recently been realized. Only a few examples of a vertical superconducting diode effect have been reported and its mechanism, especially whether intrinsic or extrinsic, remains elusive. Here we demonstrate a substantial supercurrent non-reciprocity in a van der Waals vertical Josephson junction formed with a Td-WTe2 barrier and NbSe2 electrodes that clearly reflects the intrinsic crystal structure of Td-WTe2. The Josephson diode efficiency increases with the Td-WTe2 thickness up to critical thickness, and all junctions, irrespective of the barrier thickness, reveal magneto-chiral characteristics with respect to a mirror plane of Td-WTe2. Our results, together with the twist-angle-tuned magneto-chirality of a Td-WTe2 double-barrier junction, show that two-dimensional materials promise vertical Josephson diodes with high efficiency and tunability.

Date: 2024
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DOI: 10.1038/s41467-024-45298-9

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