Stress-induced ordering evolution of 1D segmented heteronanostructures and their chemical post-transformations

Qing-Xia Chen, Yu-Yang Lu, Yang Yang, Li-Ge Chang, Yi Li, Yuan Yang, Zhen He, Jian-Wei Liu (), Yong Ni () and Shu-Hong Yu ()
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Qing-Xia Chen: University of Science and Technology of China
Yu-Yang Lu: University of Science and Technology of China
Yang Yang: University of Science and Technology of China
Li-Ge Chang: University of Science and Technology of China
Yi Li: University of Science and Technology of China
Yuan Yang: University of Science and Technology of China
Zhen He: University of Science and Technology of China
Jian-Wei Liu: University of Science and Technology of China
Yong Ni: University of Science and Technology of China
Shu-Hong Yu: University of Science and Technology of China

Nature Communications, 2024, vol. 15, issue 1, 1-12

Abstract: Abstract Investigations of one-dimensional segmented heteronanostructures (1D-SHs) have recently attracted much attention due to their potentials for applications resulting from their structure and synergistic effects between compositions and interfaces. Unfortunately, developing a simple, versatile and controlled synthetic method to fabricate 1D-SHs is still a challenge. Here we demonstrate a stress-induced axial ordering mechanism to describe the synthesis of 1D-SHs by a general under-stoichiometric reaction strategy. Using the continuum phase-field simulations, we elaborate a three-stage evolution process of the regular segment alternations. This strategy, accompanied by easy chemical post-transformations, enables to synthesize 25 1D-SHs, including 17 nanowire-nanowire and 8 nanowire-nanotube nanostructures with 13 elements (Ag, Te, Cu, Pt, Pb, Cd, Sb, Se, Bi, Rh, Ir, Ru, Zn) involved. This ordering evolution-driven synthesis will help to investigate the ordering reconstruction and potential applications of 1D-SHs.

Date: 2024
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DOI: 10.1038/s41467-024-47446-7

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