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A general finite-gel strategy for highly concentrated liquid metal inks

Ruiyu Ma, Lichuan Jia (), Zhiguang Guo, Jie Lin, Mengxin Liu, Zhixing Wang, Guilin Song, Dingxiang Yan () and Zhongming Li ()
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Ruiyu Ma: Sichuan University
Lichuan Jia: Sichuan University
Zhiguang Guo: Sichuan University
Jie Lin: Sichuan University
Mengxin Liu: Sichuan University
Zhixing Wang: Sichuan University
Guilin Song: Sichuan University
Dingxiang Yan: Sichuan University
Zhongming Li: Sichuan University

Nature Communications, 2025, vol. 16, issue 1, 1-12

Abstract: Abstract Producing high-concentration liquid metal (LM) inks is highly desirable for next-generation flexible electronics, and yet remains a dulling challenging due to the large surface tension and high density of LM droplets. Herein, a general finite-gel strategy is proposed to enable the fabrication of high-concentration liquid metal (LM) inks. In the LM-based inks, the LM droplets are confined in the relaxed finite-gel networks, which provide strong repulsive effects to avoid the reunition of the adjacent LM droplets. The unique structure imparts the LM-based inks with a good colloidal stability even at a very high LM concentration of 30,000.0 g/L. The LM-based inks also present tunable rheological behavior and are suitable for various processing technologies. Moreover, the proposed finite-gel strategy is scalable, and could be expanded to various cryogel systems (e.g., curdlan, gelatin, and gellan gum). This work takes a crucial step forward to producing highly concentrated LM-based inks for flexible electronics.

Date: 2025
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DOI: 10.1038/s41467-025-63433-y

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