Renewable diesel blendstocks produced by hydrothermal liquefaction of wet biowaste

Wan-Ting Chen, Yuanhui Zhang (), Timothy H. Lee, Zhenwei Wu, Buchun Si, Chia-Fon F. Lee, Alice Lin and Brajendra K. Sharma
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Wan-Ting Chen: University of Illinois at Urbana-Champaign
Yuanhui Zhang: University of Illinois at Urbana-Champaign
Timothy H. Lee: University of Illinois at Urbana-Champaign
Zhenwei Wu: University of Illinois at Urbana-Champaign
Buchun Si: University of Illinois at Urbana-Champaign
Chia-Fon F. Lee: University of Illinois at Urbana-Champaign
Alice Lin: University of Illinois at Urbana-Champaign
Brajendra K. Sharma: University of Illinois at Urbana-Champaign

Nature Sustainability, 2018, vol. 1, issue 11, 702-710

Abstract: Abstract Processing wet biowaste to create a useful product, a practice called valorization, is environmentally sustainable and has the potential to augment energy production. Biocrude converted from wet biowaste using hydrothermal liquefaction (HTL) has comparable heating values to petroleum crude. However, its composition is too complex for use as transportation fuels. Here, we show that distillation combined with esterification can effectively upgrade HTL biocrude oil into diesel blendstock. We demonstrate that the HTL biocrude oil converted from food processing waste and animal manure can be distilled into fractions with similar energy content to that of petroleum diesel. We then reduce the acidity of distillates through esterification to meet the diesel standard. Engine tests performed using 10–20% upgraded distillates blended with diesel show 96–100% power output, 101–102% NOx, 89–91% CO, 92–125% unburned hydrocarbon and 109–115% soot emissions, compared with regular diesel. HTL integrated with distillation and esterification has a higher energy recovery ratio than anaerobic digestion, lipid extraction, HTL combined with hydrotreating and producing diesel from petroleum. This approach realizes the potential of wet biowaste to alleviate petroleum consumption and to reduce greenhouse gas emissions.

Date: 2018
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DOI: 10.1038/s41893-018-0172-3

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