Vertical distribution of radionuclides in soil at the Semipalatinsk Test Site beyond its test locations

Andrey Panitskiy, Yelena Syssoeva, Symbat Baigazy, Assiya Kunduzbayeva, Laura Kenzhina, Yelena Polivkina, Natalya Larionova, Pavel Krivitskiy and Almira Aidarkhanova

PLOS ONE, 2023, vol. 18, issue 1, 1-12

Abstract: Data on the vertical distribution of radionuclides in the soil is necessary to fully understand the radioecological situation around ecosystems, give predictive estimates to how safe crop products are and justify a rehabilitation strategy for radioactively contaminated areas. A study was conducted to investigate the vertical distribution of radionuclides in soils of the former Semipalatinsk Test Site (STS) territory beyond its testing sites, that is, in areas in which no nuclear weapons or nuclear effects of radiological warfare agents were tested. Soil was sampled layerwise all over the Semipalatinsk Test Site down to 30 cm deep at a 5-cm spacing. Most of high activity concentrations of radionuclides all over the study area were detected in the 0–5 cm soil layer. Activity concentrations of the major man-made radionuclides were determined in soil samples collected by γ-, β and α-spectrometry. As a result, ranges of activity concentrations of 137Cs, 241Am, 90Sr and 239+240Pu were determined in 0–5, 5–10, 10–15, 15–20, 20–25, 25–30 cm soil layers. In the conventionally ‘background’ area, the 0–5 cm soil layer, on average, contains (the percentage of total activity concentration across the soil profile depth): 137Cs– 83%, 239+240Pu– 87% and 90Sr– 38%. For the 1953 plume, these values were 92%, 83% and 73%, respectively. Values for the 1951 plume in the 0–5 cm soil layer were: 137Cs– 93%, 239+240Pu– 93% and 90Sr– 59%. The minimum concentration of radionuclides are observed 20–30 cm deep in all areas studied. 90Sr is the most mobile radionuclide from the perspective of its ability to travel deep down the soil. The study found out that the nuclide vertical migration rates downward in soils based on detected activity were as follows (in descending order): 90Sr– 137Cs– 239+240Pu– 241Am. Coefficients that determine the ratio of the activity concentration of the radionuclide in the 0–20 and 0–30 cm soil cover layers to that of this radionuclide in the 0–5 cm topsoil were calculated. These coefficients enable to estimate the radionuclide inventory at each soil sampling point from their activity concentration in the 0–5 cm soil layer.

Date: 2023
References: View complete reference list from CitEc
Citations:

Downloads: (external link)
https://journals.plos.org/plosone/article?id=10.1371/journal.pone.0278581 (text/html)
https://journals.plos.org/plosone/article/file?id= ... 78581&type=printable (application/pdf)

Related works:
This item may be available elsewhere in EconPapers: Search for items with the same title.

Export reference: BibTeX RIS (EndNote, ProCite, RefMan) HTML/Text

Persistent link: https://EconPapers.repec.org/RePEc:plo:pone00:0278581

DOI: 10.1371/journal.pone.0278581

Access Statistics for this article

More articles in PLOS ONE from Public Library of Science
Bibliographic data for series maintained by plosone ().