Cycle design and optimization of pressure swing adsorption cycles for pre-combustion CO2 capture

Sai Gokul Subraveti, Kasturi Nagesh Pai, Ashwin Kumar Rajagopalan, Nicholas Stiles Wilkins, Arvind Rajendran, Ambalavan Jayaraman and Gokhan Alptekin

Applied Energy, 2019, vol. 254, issue C

Abstract: Novel pressure-swing adsorption (PSA) cycles were developed based on patented TDA AMS-19 (activated carbon) adsorbent for pre-combustion CO2 capture in integrated gasification combined cycle (IGCC) power plants. A variety of cycles comprising of counter-current blowdown, pressure equalization, steam purge and light product pressurization steps were designed and simulated using an in-house one dimensional detailed model. Full process optimization studies were performed for all cycles to evaluate their feasibility for pre-combustion CO2 capture. The CO2 purity and recovery Pareto fronts obtained using the multi-objective optimization were used to assess their ability to simultaneously achieve high CO2 purity (>95%) and recovery (>90%). The cycles that achieved the purity-recovery (95–90%) requirements were subjected to energy-productivity optimizations under the constraints of CO2 purity and recovery. Three cycle designs were ranked in terms of lowest energy consumption at 95% CO2 purities and 90% CO2 recoveries. It was found that a 10-step cycle with three pressure equalization steps achieved a minimum energy consumption of 95.7 kWhe/tonne of CO2 captured at a productivity of 3.3 mol CO2 captured/m3 adsorbent/s.

Keywords: Pre-combustion carbon capture; Pressure swing adsorption; Multi-objective optimization; Modeling; Genetic algorithm; Dynamic simulation (search for similar items in EconPapers)
Date: 2019
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Citations: View citations in EconPapers (6)

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DOI: 10.1016/j.apenergy.2019.113624

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