Optimizing H2 production from biomass: A machine learning-enhanced model of supercritical water gasification dynamics

Chengwei Huang, Jialing Xu, Shuai Xu, Murong Shan, Shanke Liu and Lijun Yu

Energy, 2024, vol. 312, issue C

Abstract: Supercritical water gasification (SCWG) is recognized as an efficient technology for biomass conversion, demonstrating substantial potential in the sustainable energy sector. This paper focuses on the H2 production by SCWG of biomass. The objective is to develop an accurate gasification kinetic model that can facilitate the optimization of industrial reactor designs. A series of SCWG experiments is conducted in a batch reactor system under temperature of 500–600 °C and residence time of 1–20 min. Based on the experimental results, a hybrid-driven model for SCWG reaction is established. Firstly, experimental data is utilized to delineate SCWG reaction mechanistic model and forecast gas yields with an acceptable error margin. Subsequently, a Wasserstein Generative Adversarial Network Gradient Boosting Regression Grid Search (WGAN-GBR-GRID) model is applied to acquire knowledge of the predictive errors from the mechanistic model and to develop a hybrid model. The hybrid-driven model significantly enhances the average relative prediction error from 15.56 % to 0.02 % when compared to the mechanistic model. This result underscores the potential of the hybrid model in optimizing SCWG technology and the Shapley Additive exPlanations (SHAP) values in feature analysis shows the possible shortcomings of mechanistic model, thereby providing a new perspective for SCWG reaction dynamics modeling.

Keywords: Supercritical water gasification; H2 production; Reaction pathway; Kinetics modeling; Hybrid modeling (search for similar items in EconPapers)
Date: 2024
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Persistent link: https://EconPapers.repec.org/RePEc:eee:energy:v:312:y:2024:i:c:s0360544224032663

DOI: 10.1016/j.energy.2024.133490

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