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Nonlinear and stochastic modelling of energy transfer in Scheibe aggregates

K.Ø. Rasmussen, Yu.B. Gaididei, O. Bang and P.L. Christiansen

Mathematics and Computers in Simulation (MATCOM), 1996, vol. 40, issue 3, 339-358

Abstract: The oxacyanine Scheibe aggregate is modelled by a two-dimensional cubic nonlinear Schrödinger equation with multiplicative noise, accounting for thermal fluctuations. For a possible choice of the physical parameters collapse of the initial state representing the Möbius-Kuhn coherent exciton may occur. The collapse time then increases with temperature. From experimental observations Möbius and Kuhn find a lifetime of the exciton which also increases with temperature. We finally consider soliton motion close to an impurity representing the acceptor molecule in the Scheibe aggregate.

Date: 1996
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Persistent link: https://EconPapers.repec.org/RePEc:eee:matcom:v:40:y:1996:i:3:p:339-358

DOI: 10.1016/0378-4754(95)00042-9

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