Cooperative and interference effects in the resonance fluorescence of two identical three-level atoms at high photon densities

Constantine Mavroyannis

Physica A: Statistical Mechanics and its Applications, 1982, vol. 110, issue 3, 431-450

Abstract: The excitation spectrum of two identical three-level atoms is considered when a strong electromagnetic field operates resonantly between two levels of the atoms. While undergoing the transition into the excited state, the atoms interact through their dipole-dipole interaction and radiate to each other as well, and subsequently, they decay radiatively into another excited state. For such a system, the spectral functions are calculated describing the cooperative and interference spectra for the symmetric and antisymmetric modes arising from the decay of the atoms from one excited state into another. In the absence of the pump field, the spectral function for the symmetric modes consists of two peaks, which are described by Lorentzian lines peaked at the frequencies ω = ω23 + VAB and ω = ω23 − VAB and having spectral widths of the order of γ021 + γ023 and γ023, respectively, where ω23 is the transition frequency between the two excited states, VAB is the dipole-dipole interaction and 12γ021 is the natural width for a photon spontaneously emitted from the 2 → 1 transition of an isolated atom. The splitting of the central peak for the transition in question and the broadening of the spectral widths are due entirely to the dipole-dipole and radiative interactions between the atoms. The spectral function for the antisymmetric modes describes a stable mode at the frequency ω = ω23 − VAB, which has a delta-function distribution, and a Lorentzian line peaked at the frequency ω = ω23 + VAB and has a spectral width of the order of γ021. In the presence of the pump field, the spectral function for the symmetric modes contains, in addition to the central peaks, two pairs of sidebands, one pair of which is induced by the pump field with an energy shift equal to Ωa/√2, while the other pair of sidebands is due to the dipole-dipole interaction between the atoms; the probability of occurrence of the latter pair of sidebands is proportional to VAB/Ωa, while the induced energy shift is equal to 3Ωa/√2, where √2Ωa is the induced by the laser field energy shift (Rabi frequency) for a single two-level atom. The spectral widths for both pairs of sidebands are of the order of γ021 + γ023. The excitation spectrum of the antisymmetric modes consists of, in addition to the central peaks, a pair of stable sidebands, which have delta-function distributions, and two pairs of sidebands, which are similar but sharper than those for the symmetric modes. Detail comparisons are given between the one- and two-atom excitation spectra for the systems under investigation.

Date: 1982
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Persistent link: https://EconPapers.repec.org/RePEc:eee:phsmap:v:110:y:1982:i:3:p:431-450

DOI: 10.1016/0378-4371(82)90061-9

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