Island coarsening in one-dimensional models with partially and completely reversible aggregation

Anna Chame and F.D.A. Aarão Reis

Physica A: Statistical Mechanics and its Applications, 2007, vol. 376, issue C, 108-116

Abstract: Using computer simulations and scaling ideas, we study one-dimensional models of diffusion, aggregation and detachment of particles from islands in the post-deposition regime, i.e., without flux. The diffusion of isolated particles takes place with unit rate, aggregation occurs immediately upon contact with another particle or island, and detachment from an island occurs with rate ε=exp(-E/kT), where E is the related energy barrier. In the partially reversible model, dissociation is limited to islands of size larger than a critical value i, while in the completely reversible model there is no restriction to that process (infinite i). Extending previous simulation results for the completely reversible case, we observe that a peaked island size distribution in the intermediate time regime, in which the mean island size is increasing, crosses over to the theoretically predicted exponentially decreasing distribution at long times. It contrasts with the partially reversible model, in which peaked distributions are obtained until the long time frozen state, which is attained with a crossover time τ∼i3/ε. The mean island size at saturation varies as Ssat≈2i+Cε (C constant), while the completely reversible case shows an Arrhenius dependence of the mean island size, S∼ε-1/2. Thus, for different coverages, the effect of the critical size i on the geometric features is much stronger than that of ε, which may be used to infer the relevance of size-dependent detachment rates in real systems and other models.

Keywords: Island coarsening; Reversible aggregation; Critical size; Scaling; Size distributions (search for similar items in EconPapers)
Date: 2007
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Persistent link: https://EconPapers.repec.org/RePEc:eee:phsmap:v:376:y:2007:i:c:p:108-116

DOI: 10.1016/j.physa.2006.10.096

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