Ferromagnetism in one-dimensional monatomic metal chains
P. Gambardella (),
A. Dallmeyer,
K. Maiti,
M. C. Malagoli,
W. Eberhardt,
K. Kern and
C. Carbone
Additional contact information
P. Gambardella: Institut de Physique des Nanostructures, EPF-Lausanne
A. Dallmeyer: Institut für Festkörperforschung, Forschungszentrum Jülich
K. Maiti: Institut für Festkörperforschung, Forschungszentrum Jülich
M. C. Malagoli: Institut für Festkörperforschung, Forschungszentrum Jülich
W. Eberhardt: Institut für Festkörperforschung, Forschungszentrum Jülich
K. Kern: Institut de Physique des Nanostructures, EPF-Lausanne
C. Carbone: Institut für Festkörperforschung, Forschungszentrum Jülich
Nature, 2002, vol. 416, issue 6878, 301-304
Abstract:
Abstract Two-dimensional systems, such as ultrathin epitaxial films and superlattices, display magnetic properties distinct from bulk materials1. A challenging aim of current research in magnetism is to explore structures of still lower dimensionality2,3,4,5,6. As the dimensionality of a physical system is reduced, magnetic ordering tends to decrease as fluctuations become relatively more important7. Spin lattice models predict that an infinite one-dimensional linear chain with short-range magnetic interactions spontaneously breaks up into segments with different orientation of the magnetization, thereby prohibiting long-range ferromagnetic order at a finite temperature7,8,9. These models, however, do not take into account kinetic barriers to reaching equilibrium or interactions with the substrates that support the one-dimensional nanostructures. Here we demonstrate the existence of both short- and long-range ferromagnetic order for one-dimensional monatomic chains of Co constructed on a Pt substrate. We find evidence that the monatomic chains consist of thermally fluctuating segments of ferromagnetically coupled atoms which, below a threshold temperature, evolve into a ferromagnetic long-range-ordered state owing to the presence of anisotropy barriers. The Co chains are characterized by large localized orbital moments and correspondingly large magnetic anisotropy energies compared to two-dimensional films and bulk Co.
Date: 2002
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DOI: 10.1038/416301a
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