Single spin detection by magnetic resonance force microscopy

D. Rugar (), R. Budakian, H. J. Mamin and B. W. Chui
Additional contact information
D. Rugar: Almaden Research Center
R. Budakian: Almaden Research Center
H. J. Mamin: Almaden Research Center
B. W. Chui: Almaden Research Center

Nature, 2004, vol. 430, issue 6997, 329-332

Abstract: Abstract Magnetic resonance imaging (MRI) is well known as a powerful technique for visualizing subsurface structures with three-dimensional spatial resolution. Pushing the resolution below 1?µm remains a major challenge, however, owing to the sensitivity limitations of conventional inductive detection techniques. Currently, the smallest volume elements in an image must contain at least 1012 nuclear spins for MRI-based microscopy1, or 107 electron spins for electron spin resonance microscopy2. Magnetic resonance force microscopy (MRFM) was proposed as a means to improve detection sensitivity to the single-spin level, and thus enable three-dimensional imaging of macromolecules (for example, proteins) with atomic resolution3,4. MRFM has also been proposed as a qubit readout device for spin-based quantum computers5,6. Here we report the detection of an individual electron spin by MRFM. A spatial resolution of 25?nm in one dimension was obtained for an unpaired spin in silicon dioxide. The measured signal is consistent with a model in which the spin is aligned parallel or anti-parallel to the effective field, with a rotating-frame relaxation time of 760?ms. The long relaxation time suggests that the state of an individual spin can be monitored for extended periods of time, even while subjected to a complex set of manipulations that are part of the MRFM measurement protocol.

Date: 2004
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DOI: 10.1038/nature02658

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