Control of four stereocentres in a triple cascade organocatalytic reaction

Dieter Enders (), Matthias R. M. Hüttl, Christoph Grondal and Gerhard Raabe
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Dieter Enders: RWTH Aachen University
Matthias R. M. Hüttl: RWTH Aachen University
Christoph Grondal: RWTH Aachen University
Gerhard Raabe: RWTH Aachen University

Nature, 2006, vol. 441, issue 7095, 861-863

Abstract: Development of an asymmetric organocatalytic triple cascade able to synthesize tetra-substituted cyclohexene carbaldehydes proceeds through a Michael/Michael/aldol condensation sequence, generating four stereogenic centres with high diastereo- and complete enantiocontrol in good to moderate yields.

Date: 2006
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DOI: 10.1038/nature04820

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