Pulsed electron paramagnetic resonance spectroscopy powered by a free-electron laser

S. Takahashi, L.-C. Brunel, D. T. Edwards, J. van Tol, G. Ramian, S. Han and M. S. Sherwin ()
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S. Takahashi: University of Southern California
L.-C. Brunel: Institute for Terahertz Science and Technology, University of California
D. T. Edwards: University of California
J. van Tol: National High Magnetic Field Laboratory, Florida State University
G. Ramian: Institute for Terahertz Science and Technology, University of California
S. Han: Institute for Terahertz Science and Technology, University of California
M. S. Sherwin: Institute for Terahertz Science and Technology, University of California

Nature, 2012, vol. 489, issue 7416, 409-413

Abstract: A free-electron laser is used to power a pulsed electron paramagnetic resonance spectrometer at 240 GHz, demonstrating a range of experimental possibilities such as the manipulation of spin-1/2 systems with 6-ns pulses and the measurement of ultrashort decoherence times.

Date: 2012
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DOI: 10.1038/nature11437

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