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Chemical mapping of a single molecule by plasmon-enhanced Raman scattering

R. Zhang, Y. Zhang, Z. C. Dong (), S. Jiang, C. Zhang, L. G. Chen, L. Zhang, Y. Liao, J. Aizpurua, Y. Luo, J. L. Yang and J. G. Hou ()
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R. Zhang: Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China
Y. Zhang: Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China
Z. C. Dong: Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China
S. Jiang: Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China
C. Zhang: Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China
L. G. Chen: Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China
L. Zhang: Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China
Y. Liao: Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China
J. Aizpurua: Material Physics Center CSIC-UPV/EHU and Donostia International Physics Center DIPC, Paseo Manuel de Lardizabal 5, Donostia-San Sebastián 20018, Spain
Y. Luo: Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China
J. L. Yang: Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China
J. G. Hou: Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China

Nature, 2013, vol. 498, issue 7452, 82-86

Abstract: Chemical mapping of a single molecule by optical means down to subnanometre resolution is achieved by spectrally matching the resonance of a nanocavity plasmon to the vibronic transitions of the molecules being studied, using tip-enhanced Raman scattering.

Date: 2013
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DOI: 10.1038/nature12151

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