Approaching disorder-free transport in high-mobility conjugated polymers

Deepak Venkateshvaran, Mark Nikolka, Aditya Sadhanala, Vincent Lemaur, Mateusz Zelazny, Michal Kepa, Michael Hurhangee, Auke Jisk Kronemeijer, Vincenzo Pecunia, Iyad Nasrallah, Igor Romanov, Katharina Broch, Iain McCulloch, David Emin, Yoann Olivier, Jerome Cornil, David Beljonne and Henning Sirringhaus ()
Additional contact information
Deepak Venkateshvaran: Optoelectronics Group, Cavendish Laboratory, University of Cambridge, JJ Thomson Avenue, Cambridge CB3 0HE, UK
Mark Nikolka: Optoelectronics Group, Cavendish Laboratory, University of Cambridge, JJ Thomson Avenue, Cambridge CB3 0HE, UK
Aditya Sadhanala: Optoelectronics Group, Cavendish Laboratory, University of Cambridge, JJ Thomson Avenue, Cambridge CB3 0HE, UK
Vincent Lemaur: Laboratory for Chemistry of Novel Materials, Université de Mons, 20 Place du Parc, 7000 Mons, Belgium
Mateusz Zelazny: Optoelectronics Group, Cavendish Laboratory, University of Cambridge, JJ Thomson Avenue, Cambridge CB3 0HE, UK
Michal Kepa: Centre for Science at Extreme Conditions, University of Edinburgh, Mayfield Road, Edinburgh EH9 3JZ, UK
Michael Hurhangee: Imperial College London, London SW7 2AZ, UK
Auke Jisk Kronemeijer: Optoelectronics Group, Cavendish Laboratory, University of Cambridge, JJ Thomson Avenue, Cambridge CB3 0HE, UK
Vincenzo Pecunia: Optoelectronics Group, Cavendish Laboratory, University of Cambridge, JJ Thomson Avenue, Cambridge CB3 0HE, UK
Iyad Nasrallah: Optoelectronics Group, Cavendish Laboratory, University of Cambridge, JJ Thomson Avenue, Cambridge CB3 0HE, UK
Igor Romanov: Optoelectronics Group, Cavendish Laboratory, University of Cambridge, JJ Thomson Avenue, Cambridge CB3 0HE, UK
Katharina Broch: Optoelectronics Group, Cavendish Laboratory, University of Cambridge, JJ Thomson Avenue, Cambridge CB3 0HE, UK
Iain McCulloch: Imperial College London, London SW7 2AZ, UK
David Emin: University of New Mexico, 1919 Lomas Boulevard Northeast, Albuquerque, New Mexico 87131, USA
Yoann Olivier: Laboratory for Chemistry of Novel Materials, Université de Mons, 20 Place du Parc, 7000 Mons, Belgium
Jerome Cornil: Laboratory for Chemistry of Novel Materials, Université de Mons, 20 Place du Parc, 7000 Mons, Belgium
David Beljonne: Laboratory for Chemistry of Novel Materials, Université de Mons, 20 Place du Parc, 7000 Mons, Belgium
Henning Sirringhaus: Optoelectronics Group, Cavendish Laboratory, University of Cambridge, JJ Thomson Avenue, Cambridge CB3 0HE, UK

Nature, 2014, vol. 515, issue 7527, 384-388

Abstract: Measurements and simulations of several high-mobility conjugated polymers show that their charge transport properties reflect an almost complete lack of disorder in the polymers, despite their amorphous microstructures, resulting from the resilience of the planar polymer backbone conformations to side-chain disorder.

Date: 2014
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DOI: 10.1038/nature13854

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