Uranium-mediated electrocatalytic dihydrogen production from water

Dominik P. Halter, Frank W. Heinemann, Julien Bachmann and Karsten Meyer ()
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Dominik P. Halter: Inorganic Chemistry, Friedrich-Alexander University Erlangen-Nürnberg (FAU)
Frank W. Heinemann: Inorganic Chemistry, Friedrich-Alexander University Erlangen-Nürnberg (FAU)
Julien Bachmann: Inorganic Chemistry, Friedrich-Alexander University Erlangen-Nürnberg (FAU)
Karsten Meyer: Inorganic Chemistry, Friedrich-Alexander University Erlangen-Nürnberg (FAU)

Nature, 2016, vol. 530, issue 7590, 317-321

Abstract: Homogenous electrocatalytic water reduction with formation of dihydrogen is demonstrated with a trisaryloxide U(III) complex, for which the catalytic cycle was elucidated and found to involve rare terminal U(iv)–OH and U(v)=O complexes.

Date: 2016
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DOI: 10.1038/nature16530

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