A pressure-amplifying framework material with negative gas adsorption transitions

Simon Krause, Volodymyr Bon, Irena Senkovska, Ulrich Stoeck, Dirk Wallacher, Daniel M. Többens, Stefan Zander, Renjith S. Pillai, Guillaume Maurin, François-Xavier Coudert and Stefan Kaskel ()
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Simon Krause: Technische Universität Dresden
Volodymyr Bon: Technische Universität Dresden
Irena Senkovska: Technische Universität Dresden
Ulrich Stoeck: Technische Universität Dresden
Dirk Wallacher: Helmholtz-Zentrum Berlin für Materialien und Energie
Daniel M. Többens: Department Structure and Dynamics of Energy Materials
Stefan Zander: Department Structure and Dynamics of Energy Materials
Renjith S. Pillai: Institut Charles Gerhardt Montpellier UMR 5253 CNRS UM ENSCM, Université Montpellier, Place E. Bataillon, 34095
Guillaume Maurin: Institut Charles Gerhardt Montpellier UMR 5253 CNRS UM ENSCM, Université Montpellier, Place E. Bataillon, 34095
François-Xavier Coudert: Chimie ParisTech, PSL Research University, CNRS, Institut de Recherche de Chimie Paris
Stefan Kaskel: Technische Universität Dresden

Nature, 2016, vol. 532, issue 7599, 348-352

Abstract: For adsorption processes, gas uptake usually increases with increasing pressure; however, here the phenomenon of negative gas adsorption is demonstrated in a metal–organic framework, which undergoes a sudden hysteretic structural deformation and pore contraction, releasing guest molecules.

Date: 2016
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DOI: 10.1038/nature17430

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