Scalable and sustainable electrochemical allylic C–H oxidation

Evan J. Horn, Brandon R. Rosen, Yong Chen, Jiaze Tang, Ke Chen, Martin D. Eastgate and Phil S. Baran ()
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Evan J. Horn: The Scripps Research Institute
Brandon R. Rosen: The Scripps Research Institute
Yong Chen: Asymchem Life Science (Tianjin), Tianjin Economic-Technological Development Zone
Jiaze Tang: Asymchem Life Science (Tianjin), Tianjin Economic-Technological Development Zone
Ke Chen: Chemical Development, Bristol–Myers Squibb
Martin D. Eastgate: Chemical Development, Bristol–Myers Squibb
Phil S. Baran: The Scripps Research Institute

Nature, 2016, vol. 533, issue 7601, 77-81

Abstract: An electrochemical C–H oxidation strategy that exhibits broad substrate scope, operational simplicity and high chemoselectivity is described; it uses inexpensive and readily available materials and represents a scalable allylic C–H oxidation that could be adopted in large-scale industrial settings without substantial environmental impact.

Date: 2016
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DOI: 10.1038/nature17431

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