Single-molecule strong coupling at room temperature in plasmonic nanocavities

Rohit Chikkaraddy, Bart de Nijs, Felix Benz, Steven J. Barrow, Oren A. Scherman, Edina Rosta, Angela Demetriadou, Peter Fox, Ortwin Hess and Jeremy J. Baumberg ()
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Rohit Chikkaraddy: NanoPhotonics Centre, Cavendish Laboratory, University of Cambridge
Bart de Nijs: NanoPhotonics Centre, Cavendish Laboratory, University of Cambridge
Felix Benz: NanoPhotonics Centre, Cavendish Laboratory, University of Cambridge
Steven J. Barrow: Melville Laboratory for Polymer Synthesis, University of Cambridge
Oren A. Scherman: Melville Laboratory for Polymer Synthesis, University of Cambridge
Edina Rosta: King’s College London
Angela Demetriadou: Blackett Laboratory, Prince Consort Road, Imperial College
Peter Fox: Blackett Laboratory, Prince Consort Road, Imperial College
Ortwin Hess: Blackett Laboratory, Prince Consort Road, Imperial College
Jeremy J. Baumberg: NanoPhotonics Centre, Cavendish Laboratory, University of Cambridge

Nature, 2016, vol. 535, issue 7610, 127-130

Abstract: Placing a light emitter in an ultra-small optical cavity results in coupling between matter and light, generating new forms of emission that can be exploited in practical or fundamental applications; here, a system is described in which strong light–matter coupling occurs at room temperature and in ambient conditions by aligning single dye molecules in the optical cavities between gold nanoparticles and surfaces.

Date: 2016
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DOI: 10.1038/nature17974

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