Directed evolution of artificial metalloenzymes for in vivo metathesis

Markus Jeschek, Raphael Reuter, Tillmann Heinisch, Christian Trindler, Juliane Klehr, Sven Panke () and Thomas R. Ward ()
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Markus Jeschek: ETH Zurich
Raphael Reuter: University of Basel
Tillmann Heinisch: University of Basel
Christian Trindler: University of Basel
Juliane Klehr: University of Basel
Sven Panke: ETH Zurich
Thomas R. Ward: University of Basel

Nature, 2016, vol. 537, issue 7622, 661-665

Abstract: An artificial metalloenzyme is compartmentalized and evolved in vivo for olefin metathesis—an archetypal organometallic reaction without equivalent in nature; the evolved metathase reveals broad substrate scope and compares favourably with commercial catalysts.

Date: 2016
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DOI: 10.1038/nature19114

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