Attosecond angular streaking and tunnelling time in atomic hydrogen

U. Satya Sainadh, Han Xu (), Xiaoshan Wang, A. Atia-Tul-Noor, William C. Wallace, Nicolas Douguet, Alexander Bray, Igor Ivanov, Klaus Bartschat, Anatoli Kheifets, R. T. Sang () and I. V. Litvinyuk ()
Additional contact information
U. Satya Sainadh: Griffith University
Han Xu: Griffith University
Xiaoshan Wang: Lanzhou University
A. Atia-Tul-Noor: Griffith University
William C. Wallace: Griffith University
Nicolas Douguet: Drake University
Alexander Bray: The Australian National University
Igor Ivanov: Institute for Basic Science
Klaus Bartschat: Drake University
Anatoli Kheifets: The Australian National University
R. T. Sang: Griffith University
I. V. Litvinyuk: Griffith University

Nature, 2019, vol. 568, issue 7750, 75-77

Abstract: Abstract The tunnelling of a particle through a potential barrier is a key feature of quantum mechanics that goes to the core of wave–particle duality. The phenomenon has no counterpart in classical physics, and there are no well constructed dynamical observables that could be used to determine ‘tunnelling times’. The resulting debate1–5 about whether a tunnelling quantum particle spends a finite and measurable time under a potential barrier was reignited in recent years by the advent of ultrafast lasers and attosecond metrology6. Particularly important is the attosecond angular streaking (‘attoclock’) technique7, which can time the release of electrons in strong-field ionization with a precision of a few attoseconds. Initial measurements7–10 confirmed the prevailing view that tunnelling is instantaneous, but later studies11,12 involving multi-electron atoms—which cannot be accurately modelled, complicating interpretation of the ionization dynamics—claimed evidence for finite tunnelling times. By contrast, the simplicity of the hydrogen atom enables precise experimental measurements and calculations13–15 and makes it a convenient benchmark. Here we report attoclock and momentum-space imaging16 experiments on atomic hydrogen and compare these results with accurate simulations based on the three-dimensional time-dependent Schrödinger equation and our experimental laser pulse parameters. We find excellent agreement between measured and simulated data, confirming the conclusions of an earlier theoretical study17 of the attoclock technique in atomic hydrogen that presented a compelling argument for instantaneous tunnelling. In addition, we identify the Coulomb potential as the sole cause of the measured angle between the directions of electron emission and peak electric field: this angle had been attributed11,12 to finite tunnelling times. We put an upper limit of 1.8 attoseconds on any tunnelling delay, in agreement with recent theoretical findings18 and ruling out the interpretation of all commonly used ‘tunnelling times’19 as ‘time spent by an electron under the potential barrier’20.

Date: 2019
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DOI: 10.1038/s41586-019-1028-3

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