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Diode effect in Josephson junctions with a single magnetic atom

Martina Trahms, Larissa Melischek, Jacob F. Steiner, Bharti Mahendru, Idan Tamir, Nils Bogdanoff, Olof Peters, Gaël Reecht, Clemens B. Winkelmann, Felix Oppen and Katharina J. Franke ()
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Martina Trahms: Freie Universität Berlin
Larissa Melischek: Freie Universität Berlin
Jacob F. Steiner: Freie Universität Berlin
Bharti Mahendru: Freie Universität Berlin
Idan Tamir: Freie Universität Berlin
Nils Bogdanoff: Freie Universität Berlin
Olof Peters: Freie Universität Berlin
Gaël Reecht: Freie Universität Berlin
Clemens B. Winkelmann: Université Grenoble Alpes, CNRS, Institut Neél
Felix Oppen: Freie Universität Berlin
Katharina J. Franke: Freie Universität Berlin

Nature, 2023, vol. 615, issue 7953, 628-633

Abstract: Abstract Current flow in electronic devices can be asymmetric with bias direction, a phenomenon underlying the utility of diodes1 and known as non-reciprocal charge transport2. The promise of dissipationless electronics has recently stimulated the quest for superconducting diodes, and non-reciprocal superconducting devices have been realized in various non-centrosymmetric systems3–10. Here we investigate the ultimate limits of miniaturization by creating atomic-scale Pb–Pb Josephson junctions in a scanning tunnelling microscope. Pristine junctions stabilized by a single Pb atom exhibit hysteretic behaviour, confirming the high quality of the junctions, but no asymmetry between the bias directions. Non-reciprocal supercurrents emerge when inserting a single magnetic atom into the junction, with the preferred direction depending on the atomic species. Aided by theoretical modelling, we trace the non-reciprocity to quasiparticle currents flowing by means of electron–hole asymmetric Yu–Shiba–Rusinov states inside the superconducting energy gap and identify a new mechanism for diode behaviour in Josephson junctions. Our results open new avenues for creating atomic-scale Josephson diodes and tuning their properties through single-atom manipulation.

Date: 2023
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DOI: 10.1038/s41586-023-05743-z

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