Two-axis twisting using Floquet-engineered XYZ spin models with polar molecules
Calder Miller (),
Annette N. Carroll,
Junyu Lin,
Henrik Hirzler,
Haoyang Gao,
Hengyun Zhou,
Mikhail D. Lukin and
Jun Ye ()
Additional contact information
Calder Miller: University of Colorado
Annette N. Carroll: University of Colorado
Junyu Lin: University of Colorado
Henrik Hirzler: University of Colorado
Haoyang Gao: Harvard University
Hengyun Zhou: Harvard University
Mikhail D. Lukin: Harvard University
Jun Ye: University of Colorado
Nature, 2024, vol. 633, issue 8029, 332-337
Abstract:
Abstract Polar molecules confined in an optical lattice are a versatile platform to explore spin-motion dynamics based on strong, long-range dipolar interactions1,2. The precise tunability3 of Ising and spin-exchange interactions with both microwave and d.c. electric fields makes the molecular system particularly suitable for engineering complex many-body dynamics4–6. Here we used Floquet engineering7 to realize new quantum many-body systems of polar molecules. Using a spin encoded in the two lowest rotational states of ultracold 40K87Rb molecules, we mutually validated XXZ spin models tuned by a Floquet microwave pulse sequence against those tuned by a d.c. electric field through observations of Ramsey contrast dynamics. This validation sets the stage for the realization of Hamiltonians inaccessible with static fields. In particular, we observed two-axis twisting8 mean-field dynamics, generated by a Floquet-engineered XYZ model using itinerant molecules in two-dimensional layers. In the future, Floquet-engineered Hamiltonians could generate entangled states for molecule-based precision measurement9 or could take advantage of the rich molecular structure for quantum simulation of multi-level systems10,11.
Date: 2024
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DOI: 10.1038/s41586-024-07883-2
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