Cooperative luminescence quenching on many-particle acceptors in disordered media
T.T. Basiev and
I.T. Basieva
Physica A: Statistical Mechanics and its Applications, 2012, vol. 391, issue 12, 3526-3532
Abstract:
Many-body cooperative energy transfer is an important process in biology, medicine, photosynthesis, rare-earth-doped laser materials, responsible for up- and down-conversion of energy, optical excitation sensitization and relaxation. We present an analytical solution for long-time asymptotic of static luminescence quenching kinetics due to cooperative energy transfer to ensembles of acceptors comprised of two-, three-, and more particles. For cooperative energy transfer and cooperative luminescence quenching to n-body acceptors we have discovered a new law of power d/(nS−(n−1)d) time dependence (d=1,2,3 is the space dimension, S=6,8,10 is the multipolarty of interaction: dipole–dipole, dipole–quadrupole, or quadrupole–quadrupole). The detailed numerical simulation of cooperative quenching by Monte-Carlo method confirms the theoretical result.
Keywords: Energy transfer; Down-conversion; Rare-earth ions (search for similar items in EconPapers)
Date: 2012
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Persistent link: https://EconPapers.repec.org/RePEc:eee:phsmap:v:391:y:2012:i:12:p:3526-3532
DOI: 10.1016/j.physa.2012.02.017
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