Femtosecond response of polyatomic molecules to ultra-intense hard X-rays

A. Rudenko (), L. Inhester, K. Hanasaki, X. Li, S. J. Robatjazi, B. Erk, R. Boll, K. Toyota, Y. Hao, O. Vendrell, C. Bomme, E. Savelyev, B. Rudek, L. Foucar, S. H. Southworth, C. S. Lehmann, B. Kraessig, T. Marchenko, M. Simon, K. Ueda, K. R. Ferguson, M. Bucher, T. Gorkhover, S. Carron, R. Alonso-Mori, J. E. Koglin, J. Correa, G. J. Williams, S. Boutet, L. Young, C. Bostedt, S.-K. Son (), R. Santra and D. Rolles
Additional contact information
A. Rudenko: J. R. Macdonald Laboratory, Kansas State University
L. Inhester: Center for Free-Electron Laser Science, Deutsches Elektronen-Synchrotron (DESY)
K. Hanasaki: Center for Free-Electron Laser Science, Deutsches Elektronen-Synchrotron (DESY)
X. Li: J. R. Macdonald Laboratory, Kansas State University
S. J. Robatjazi: J. R. Macdonald Laboratory, Kansas State University
B. Erk: Deutsches Elektronen-Synchrotron (DESY)
R. Boll: Deutsches Elektronen-Synchrotron (DESY)
K. Toyota: Center for Free-Electron Laser Science, Deutsches Elektronen-Synchrotron (DESY)
Y. Hao: Center for Free-Electron Laser Science, Deutsches Elektronen-Synchrotron (DESY)
O. Vendrell: Center for Free-Electron Laser Science, Deutsches Elektronen-Synchrotron (DESY)
C. Bomme: Deutsches Elektronen-Synchrotron (DESY)
E. Savelyev: Deutsches Elektronen-Synchrotron (DESY)
B. Rudek: Physikalisch-Technische Bundesanstalt (PTB)
L. Foucar: Max Planck Institute for Medical Research
S. H. Southworth: Argonne National Laboratory
C. S. Lehmann: Argonne National Laboratory
B. Kraessig: Argonne National Laboratory
T. Marchenko: Sorbonne Universités, UPMC Université Paris 06, CNRS, LCP-MR (UMR 7614)
M. Simon: Sorbonne Universités, UPMC Université Paris 06, CNRS, LCP-MR (UMR 7614)
K. Ueda: Institute of Multidisciplinary Research for Advanced Materials, Tohoku University
K. R. Ferguson: Linac Coherent Light Source (LCLS), SLAC National Accelerator Laboratory
M. Bucher: Argonne National Laboratory
T. Gorkhover: Linac Coherent Light Source (LCLS), SLAC National Accelerator Laboratory
S. Carron: Linac Coherent Light Source (LCLS), SLAC National Accelerator Laboratory
R. Alonso-Mori: Linac Coherent Light Source (LCLS), SLAC National Accelerator Laboratory
J. E. Koglin: Linac Coherent Light Source (LCLS), SLAC National Accelerator Laboratory
J. Correa: Center for Free-Electron Laser Science, Deutsches Elektronen-Synchrotron (DESY)
G. J. Williams: Linac Coherent Light Source (LCLS), SLAC National Accelerator Laboratory
S. Boutet: Linac Coherent Light Source (LCLS), SLAC National Accelerator Laboratory
L. Young: Argonne National Laboratory
C. Bostedt: Argonne National Laboratory
S.-K. Son: Center for Free-Electron Laser Science, Deutsches Elektronen-Synchrotron (DESY)
R. Santra: Center for Free-Electron Laser Science, Deutsches Elektronen-Synchrotron (DESY)
D. Rolles: J. R. Macdonald Laboratory, Kansas State University

Nature, 2017, vol. 546, issue 7656, 129-132

Abstract: Upon exposure to ultra-intense, hard X-ray pulses, polyatomic molecules containing one heavy atom reach a much higher degree of ionization than do individual heavy atoms, contrary to previous assumptions.

Date: 2017
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DOI: 10.1038/nature22373

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